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Counties: Union County Union County Area: 162 square miles Location: Eastern Indiana, bordered on the north by Wayne County, to the east by Ohio, to the south by Franklin County, and to the west by Fayette County. Population: 7,349 (2000 Census) Cities & Towns: Liberty (county seat, 2,061, 211th largest city in the State); West College Corner (634) Named For: the Union of American States.